Functional Materials and Microsystems – Publications
Full publication list of the research group can be found in the RMIT Research Repository.
Selected recent publications
Field effect biosensing platform based on 2D α‑MoO3
S. Balendhran, S. Walia, M. Alsaif, E. P. Nguyen, J. Z. Ou, S. Zhuiykov, S. Sriram, M. Bhaskaran, and K. Kalantar-zadeh
ACS Nano Article ASAP (2013). [doi: 10.1021/nn403241f]
Abstract: Electrical-based biosensing platforms offer ease of fabrication and simple sensing solutions. Recently, two-dimensional (2D) semiconductors have been proven to be excellent for the fabrication of field effect transistors (FETs) due to their large transconductance, which can be efficiently used for developing sensitive bioplatforms. We present a 2D molybdenum trioxide (MoO3) FET based biosensing platform, using bovine serum albumin as a model protein. The conduction channel is a nanostructured film made of 2D α-MoO3 nanoflakes, with the majority of nanoflake thicknesses being equal to or less than 2.8 nm. The response time is impressively low (less than 10 s), which is due to the high permittivity of the 2D α-MoO3 nanoflakes. The system offers a competitive solution for future biosensing applications.
Transparent functional oxide stretchable electronics: Micro-tectonics enabled high strain electrodes
P. Gutruf, C. M. Shah, S. Walia, H. Nili, A. S. Zoolfakar, C. Karnutsch, K. Kalantar-zadeh, S. Sriram, and M. Bhaskaran
NPG Asia Materials 5 e62 (2013). [doi: 10.1038/am.2013.41]
Abstract: Fully transparent and flexible electronic substrates that incorporate functional materials are the precursors to realising next-generation devices with sensing, self-powering and portable functionalities. Here, we demonstrate a universal process for transferring planar, transparent functional oxide thin films on to elastomeric polydimethylsiloxane (PDMS) substrates. This process overcomes the challenge of incorporating high-temperature-processed crystalline oxide materials with low-temperature organic substrates. The functionality of the process is demonstrated using indium tin oxide (ITO) thin films to realise fully transparent and flexible resistors. The ITO thin films on PDMS are shown to withstand uniaxial strains of 15%, enabled by microstructure tectonics. Furthermore, zinc oxide was transferred to display the versatility of this transfer process. Such a ubiquitous process for the transfer of functional thin films to elastomeric substrates will pave the way for touch sensing and energy harvesting for displays and electronics with flexible and transparent characteristics.
Transition metal oxides - thermoelectric properties
S. Walia, S. Balendhran, H. Nili, S. Zhuiykov, G. Rosengarten, Q. H. Wang, M. Bhaskaran, S. Sriram, M. S. Strano, and K. Kalantar-zadeh
Progress in Materials Science (2013). [doi: 10.1016/j.pmatsci.2013.06.003]
Abstract: Transition metal oxides (TMOs) are a fascinating class of materials due to their wide ranging electronic, chemical and mechanical properties. Additionally, they are gaining increasing attention for their thermoelectric (TE) properties due to their high temperature stability, tunable electronic and phonon transport properties and well established synthesis techniques. In this article, we review TE TMOs at cryogenic, ambient and high temperatures. An overview of strategies used for morphological, composting and stoichiometric tuning of their key TE parameters is presented. This article also provides an outlook on the current and future prospects of implementing TMOs for a wide range of TE applications.
Terahertz localized surface plasmon resonances in coaxial microcavities
W. Withayachumnankul, C. M. Shah, C. Fumeaux, K. Kaltenecker, M. Walther, B. M. Fischer, D. Abbott, M. Bhaskaran, and S. Sriram
Advanced Optical Materials 1 443 (2013). [doi 10.1002/adom.201300021]
Abstract: Coaxial microcavities etched into the surface of a doped silicon substrate are shown to support localized surface plasmon resonances at terahertz frequencies. The underlying mechanism involves coupling freely propagating terahertz waves with surface plasmon polaritons (SPPs), which propagate in a coaxial mode along the cavity walls in the axial direction. A Fabry–Pérot resonance is built up when the SPP wavenumber appropriately relates to the cavity depth. Owing to the Ohmic loss of the silicon at terahertz frequencies, the energy of the resonating SPPs is largely dissipated, leading to a modified reflection spectrum. Strong field enhancement is observed inside the cavities at resonance. The theoretical analysis is supported by numerical and experimental results. This study is a promising pathway for development of terahertz devices with applications in the areas of photonic integrated circuits, molecular sensing, and subwavelength imaging.
Dielectric resonator nanoantennas at visible frequencies
L. Zou, W. Withayachumnankul, C. M. Shah, A. Mitchell, M. Bhaskaran, S. Sriram, and C. Fumeaux
Optics Express 21 1344 (2013) [doi 10.1364/OE.21.001344]
Abstract: Drawing inspiration from radio-frequency technologies, we propose a realization of nano-scale optical dielectric resonator antennas (DRAs) functioning in their fundamental mode. These DRAs operate via displacement current in a low-loss high-permittivity dielectric, resulting in reduced energy dissipation in the resonators. The designed nonuniform planar DRA array on a metallic plane imparts a sequence of phase shifts across the wavefront to create beam deflection off the direction of specular reflection. The realized array clearly demonstrates beam deflection at 633 nm. Despite the loss introduced by field interaction with the metal substrate, the proposed low-loss resonator concept is a first step towards nanoantennas with enhanced efficiency. The compact planar structure and technologically relevant materials promise monolithic circuit integration of DRAs.
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